Radiation shielding performance of (SmEuYbLaEr)2TaO4 high-entropy oxide reinforced Cu matrix composites
Özet
High-entropy oxides (HEOs) containing rare earth elements are attracting increasing interest due to their thermal stability and potential for use in radiation shielding applications. In this study, the high-entropy oxide (SmEuYbLaEr)2TaO4 was synthesized via mechanical alloying (MA) followed by calcination and incorporated into a Cu matrix at different reinforcement levels to produce volumetric composites. Structural, thermal, and microstructural analyses confirmed the successful formation of a stable HEO phase and its effective dispersion within the Cu matrix. The radiation shielding performance of the composites was experimentally evaluated over a wide range of photon energies using standard gamma-ray sources. The results showed that shielding performance depends largely on both photon energy and HEO content. Increasing the HEO concentration significantly reduced the half-value layer (HVL) while substantially increasing the mass attenuation coefficient (MAC) and radiation protection efficiency (RPE), particularly in the low- and medium-energy regions where the photoelectric effect is dominant. Among the materials studied, the Cu composite containing 20 wt% HEO exhibited the best overall shielding performance. These results demonstrate that (SmEuYbLaEr)2TaO4 is an effective additive for improving the radiation shielding capability of Cu-based composites and highlight its potential for advanced radiation protection applications.
Anahtar Kelimeler
- Scopus
- 1
- OpenAlex
- 1
Tam Kayıt
| Alan | Değer | Dil |
|---|---|---|
| dc.contributor.author | Taşgın, Yahya | |
| dc.contributor.author | Yılmaz, Demet | |
| dc.contributor.author | Kanca, M. Sait | |
| dc.contributor.author | Kök, Mediha | |
| dc.contributor.author | Yayla, Nihal | |
| dc.contributor.author | Güler, Ömer | |
| dc.date.accessioned | 2026-10-28T14:53:57.938089807Z | |
| dc.date.available | 2026-10-28T14:53:57.938089807Z | |
| dc.date.issued | 2026 | |
| dc.description.abstract | High-entropy oxides (HEOs) containing rare earth elements are attracting increasing interest due to their thermal stability and potential for use in radiation shielding applications. In this study, the high-entropy oxide (SmEuYbLaEr)2TaO4 was synthesized via mechanical alloying (MA) followed by calcination and incorporated into a Cu matrix at different reinforcement levels to produce volumetric composites. Structural, thermal, and microstructural analyses confirmed the successful formation of a stable HEO phase and its effective dispersion within the Cu matrix. The radiation shielding performance of the composites was experimentally evaluated over a wide range of photon energies using standard gamma-ray sources. The results showed that shielding performance depends largely on both photon energy and HEO content. Increasing the HEO concentration significantly reduced the half-value layer (HVL) while substantially increasing the mass attenuation coefficient (MAC) and radiation protection efficiency (RPE), particularly in the low- and medium-energy regions where the photoelectric effect is dominant. Among the materials studied, the Cu composite containing 20 wt% HEO exhibited the best overall shielding performance. These results demonstrate that (SmEuYbLaEr)2TaO4 is an effective additive for improving the radiation shielding capability of Cu-based composites and highlight its potential for advanced radiation protection applications. | |
| dc.description.sponsorship | Munzur Üniversitesi, MU, (İHTS2026-03) | |
| dc.identifier.doi | 10.1016/j.ceramint.2026.07.564 | |
| dc.identifier.issn | 0272-8842 | |
| dc.identifier.scopus | 2-s2.0-105046145875 | |
| dc.identifier.uri | https://rdlopen.rawdatalibrary.net/r/munzur/1177 | |
| dc.language.iso | en | |
| dc.publisher | Elsevier Ltd | |
| dc.relation.ispartof | Ceramics International | |
| dc.rights | info:eu-repo/semantics/openAccess | |
| dc.subject | Cu matrix composites | |
| dc.subject | Gamma attenuation | |
| dc.subject | High-entropy oxide | |
| dc.subject | Radiation shielding | |
| dc.subject.other | Copper | |
| dc.subject.other | Copper compounds | |
| dc.subject.other | Entropy | |
| dc.subject.other | Gamma rays | |
| dc.subject.other | High-entropy alloys | |
| dc.subject.other | Photoelectricity | |
| dc.subject.other | Reinforcement | |
| dc.subject.other | Tantalum compounds | |
| dc.subject.other | Cu matrix composites | |
| dc.subject.other | Gamma attenuation | |
| dc.subject.other | High-entropy oxide | |
| dc.subject.other | matrix | |
| dc.subject.other | Photon energy | |
| dc.subject.other | Rare-earths | |
| dc.subject.other | Shielding applications | |
| dc.subject.other | Shielding performance | |
| dc.subject.other | Synthesised | |
| dc.subject.other | Thermal | |
| dc.subject.other | Radiation shielding | |
| dc.title | Radiation shielding performance of (SmEuYbLaEr)2TaO4 high-entropy oxide reinforced Cu matrix composites | |
| dc.type | Article | |
| rdl.citation.openalex | 1 | |
| rdl.citation.scopus | 1 | |
| rdl.oa.status | closed | |
| rdl.oa.status | green | |
| rdl.oa.url | https://hdl.handle.net/11508/64905 | |
| rdl.publication.status | inPress | |
| rdl.scopus.quartile | Q1 | |
| rdl.source.index | SCOPUS |
