Radiation shielding performance of (SmEuYbLaEr)2TaO4 high-entropy oxide reinforced Cu matrix composites

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High-entropy oxides (HEOs) containing rare earth elements are attracting increasing interest due to their thermal stability and potential for use in radiation shielding applications. In this study, the high-entropy oxide (SmEuYbLaEr)2TaO4 was synthesized via mechanical alloying (MA) followed by calcination and incorporated into a Cu matrix at different reinforcement levels to produce volumetric composites. Structural, thermal, and microstructural analyses confirmed the successful formation of a stable HEO phase and its effective dispersion within the Cu matrix. The radiation shielding performance of the composites was experimentally evaluated over a wide range of photon energies using standard gamma-ray sources. The results showed that shielding performance depends largely on both photon energy and HEO content. Increasing the HEO concentration significantly reduced the half-value layer (HVL) while substantially increasing the mass attenuation coefficient (MAC) and radiation protection efficiency (RPE), particularly in the low- and medium-energy regions where the photoelectric effect is dominant. Among the materials studied, the Cu composite containing 20 wt% HEO exhibited the best overall shielding performance. These results demonstrate that (SmEuYbLaEr)2TaO4 is an effective additive for improving the radiation shielding capability of Cu-based composites and highlight its potential for advanced radiation protection applications.

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dc.contributor.authorTaşgın, Yahya
dc.contributor.authorYılmaz, Demet
dc.contributor.authorKanca, M. Sait
dc.contributor.authorKök, Mediha
dc.contributor.authorYayla, Nihal
dc.contributor.authorGüler, Ömer
dc.date.accessioned2026-10-28T14:53:57.938089807Z
dc.date.available2026-10-28T14:53:57.938089807Z
dc.date.issued2026
dc.description.abstractHigh-entropy oxides (HEOs) containing rare earth elements are attracting increasing interest due to their thermal stability and potential for use in radiation shielding applications. In this study, the high-entropy oxide (SmEuYbLaEr)2TaO4 was synthesized via mechanical alloying (MA) followed by calcination and incorporated into a Cu matrix at different reinforcement levels to produce volumetric composites. Structural, thermal, and microstructural analyses confirmed the successful formation of a stable HEO phase and its effective dispersion within the Cu matrix. The radiation shielding performance of the composites was experimentally evaluated over a wide range of photon energies using standard gamma-ray sources. The results showed that shielding performance depends largely on both photon energy and HEO content. Increasing the HEO concentration significantly reduced the half-value layer (HVL) while substantially increasing the mass attenuation coefficient (MAC) and radiation protection efficiency (RPE), particularly in the low- and medium-energy regions where the photoelectric effect is dominant. Among the materials studied, the Cu composite containing 20 wt% HEO exhibited the best overall shielding performance. These results demonstrate that (SmEuYbLaEr)2TaO4 is an effective additive for improving the radiation shielding capability of Cu-based composites and highlight its potential for advanced radiation protection applications.
dc.description.sponsorshipMunzur Üniversitesi, MU, (İHTS2026-03)
dc.identifier.doi10.1016/j.ceramint.2026.07.564
dc.identifier.issn0272-8842
dc.identifier.scopus2-s2.0-105046145875
dc.identifier.urihttps://rdlopen.rawdatalibrary.net/r/munzur/1177
dc.language.isoen
dc.publisherElsevier Ltd
dc.relation.ispartofCeramics International
dc.rightsinfo:eu-repo/semantics/openAccess
dc.subjectCu matrix composites
dc.subjectGamma attenuation
dc.subjectHigh-entropy oxide
dc.subjectRadiation shielding
dc.subject.otherCopper
dc.subject.otherCopper compounds
dc.subject.otherEntropy
dc.subject.otherGamma rays
dc.subject.otherHigh-entropy alloys
dc.subject.otherPhotoelectricity
dc.subject.otherReinforcement
dc.subject.otherTantalum compounds
dc.subject.otherCu matrix composites
dc.subject.otherGamma attenuation
dc.subject.otherHigh-entropy oxide
dc.subject.othermatrix
dc.subject.otherPhoton energy
dc.subject.otherRare-earths
dc.subject.otherShielding applications
dc.subject.otherShielding performance
dc.subject.otherSynthesised
dc.subject.otherThermal
dc.subject.otherRadiation shielding
dc.titleRadiation shielding performance of (SmEuYbLaEr)2TaO4 high-entropy oxide reinforced Cu matrix composites
dc.typeArticle
rdl.citation.openalex1
rdl.citation.scopus1
rdl.oa.statusclosed
rdl.oa.statusgreen
rdl.oa.urlhttps://hdl.handle.net/11508/64905
rdl.publication.statusinPress
rdl.scopus.quartileQ1
rdl.source.indexSCOPUS